Modelling the Dissociation Dynamics and Threshold Photoelectron Spectra of Small Halogenated Molecules - Jonelle Harvey  [Gebundene Ausgabe]

Modelling the Dissociation Dynamics and Threshold Photoelectron Spectra of Small Halogenated Molecules - Jonelle Harvey [Gebundene Ausgabe]

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Produktinformationen

Details
EAN / ISBN-139783319029757
Höhe23.5 cm
AutorJonelle Harvey
Produktformgebundene Ausgabe
Seitenanzahl174
HerausgeberSpringer International Publishing
Erscheinungsdatum 2013
InhaltsverzeichnisIntroduction.- Measuring the photoelectron signal.- The study of ionic dissociations.- Thermochemistry.- Experimental.- The synchrotron radiation source.- The endstation.- Capturing the electron signal.- The experimental results.- Theory.- Computational methods.- Modelling.- Fast dissociations of halogenated methanes: a thermochemical network.- Introduction.- Conclusions.- Photodissociation dynamics of four fluorinated ethenes: fast, slow, statistical and non-statistical reactions.- Introduction.- Results and Discussion.- Conclusions.- Threshold photoelectron spectra of four fluorinated ethenes from the ground electronic state to higher electronic states.- Introduction.- Results and Discussion.- Conclusions.- Conclusions and further work.- Conclusions.- Further work.- Beyond TPEPICO.- Appendices.
HauptbeschreibungJonelle Harvey's book outlines two related experimental techniques, threshold photoelectron spectroscopy and threshold photoelectron photoion coincidence techniques, which are utilised to investigate small halogenated molecules. All the experiments were conducted at the vacuum ultraviolet beamline of the Swiss Light Source, a synchrotron photon source, which has the advantage over popular laser photon-sources of extreme ease of tunability. Three studies are presented which combine experimental and computational ab initio approaches: studying the fast dissociations of halogenated methanes in order to construct a self-consistent thermochemical network; investigating the fragmentations of fluoroethenes from timebombs, which break apart very slowly but explosively, to fast dissociators; and uncovering how vital conical interactions underpin both the results of photoelectron spectra and dissociation patterns. The details included in this thesis are useful for researchers working in the same field and those readers wishing to obtain a solid introduction into the types of systems encountered in threshold photoelectron photoion coincidence spectroscopy.
Breite15.5 cm
SpracheEnglisch

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