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Bücher Wissen & Bildung Naturwissenschaft, Medizin, Informatik, Technik Physik & Astronomie Atomphysik & Kernphysik Broadband Dielectric Spectroscopy in Neat and Binary Molecular Glass Formers
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Broadband Dielectric Spectroscopy in Neat and Binary Molecular Glass Formers
Thomas Blochowicz (Broschiert, Englisch)
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Beschreibung
Neat and binary molecular glass formers are investigated by
means of broadband dielectric spectroscopy with the aim of
gaining a systematic understanding of the molecular slowing down, which
is characteristic for the glass transition. By combining frequency and
time domain techniques a dynamic range from 10⁻6 Hz up to
10 Hz is covered. Particular attention is drawn to the fact that
different types… of secondary relaxations may appear
during the process of supercooling. In certain simple glass formers such secondary
processes are clearly of intermolecular origin, and it turns out
that in mixtures of small and large molecules
secondary relaxations can be systematically altered by changing the
concentration of the constituents. Thus, the relation between
different types of secondary processes may be clarified.
It is typical of glass forming substances that the decay of orientational
correlations is non-exponential, and, correspondingly, the
dielectric loss spectra are broadened as compared to a simple Debye-like
relaxation process. The latter effect is particularly pronounced in
binary glass formers, and one aim of the present work is to provide
and apply an appropriate tool for a line shape analysis of the relaxation spectra in
both neat end binary systems. On the other hand, the nature of
spectral broadening is investigated by means of non-resonant
dielectric hole burning, which allows to distinguish
between heterogeneous and homogeneous dynamics in a system. It turns out that inbinary glass formers dynamic heterogeneities are particularly pronounced and
that the effects of dielectric hole burning in both neat and binary
systems are very well described within the framework of a model of
selective local heating. Dieses Produkt haben wir gerade leider nicht auf Lager.
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Technische Daten
Erscheinungsdatum
25.08.2003
Sprache
Englisch
EAN
9783832503208
Herausgeber
Logos Berlin
Sonderedition
Nein
Autor
Thomas Blochowicz
Seitenanzahl
241
Auflage
1
Einbandart
Broschiert
Buch Untertitel
Frequency and Time Domain Spectroscopy, Non-Resonant Spectral Hole Burning
Schlagwörter
Glasübergang, Lochbrennspektroskopie, binäre Glasbildner, dielektrische Spektroskopie
Höhe
210 mm
Breite
14.5 cm
-.-
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